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Wednesday, 2 September 2015

Fifteen-year trends in criteria air pollutants in oil sands communities of Alberta, Canada


Highlights

Small increasing trends were observed for NO2 at two oil sands communities.
No meaningful trends occurred for SO2 at all oil sands communities.
No notable trends were observed for O3, PM2.5, and CO over the 15-year period.
No indications of air quality trends were found at Fort Chipewyan.
Forest fire smoke plays a key role for PM2.5 exceedances at all communities.

Abstract

An investigation of ambient air quality was undertaken at three communities within the Athabasca Oil Sands Region (AOSR) of Alberta, Canada (Fort McKay, Fort McMurray, and Fort Chipewyan). Daily and seasonal patterns and 15-year trends were investigated for several criteria air pollutants over the period of 1998 to 2012. A parametric trend detection method using percentiles from frequency distributions of 1 h concentrations for a pollutant during each year was used. Variables representing 50th, 65th, 80th, 90th, 95th and 98th percentile concentrations each year were identified from frequency distributions and used for trend analysis. Small increasing concentration trends were observed for nitrogen dioxide (< 1 ppb/year) at Fort McKay and Fort McMurray over the period consistent with increasing emissions of oxides of nitrogen (ca. 1000 tons/year) from industrial developments. Emissions from all oil sands facilities appear to be contributing to the trend at Fort McKay, whereas both emissions from within the community (vehicles and commercial) and oil sands facility emissions appear to be contributing to the trend at Fort McMurray. Sulfur dioxide (SO2) emissions from industrial developments in the AOSR were unchanged during the period (101,000 ± 7000 tons/year; mean ± standard deviation) and no meaningful trends were judged to be occurring at all community stations. No meaningful trends occurred for ozone and fine particulate matter (PM2.5) at all community stations and carbon monoxide at one station in Fort McMurray. Air quality in Fort Chipewyan was much better and quite separate in terms of absence of factors influencing criteria air pollutant concentrations at the other community stations.

Keywords

  • Alberta's oil sands; 
  • Air quality; 
  • Trends; 
  • Fort McKay; 
  • Fort McMurray; 
  • Fort Chipewyan

Corresponding author. Tel.:+1 780 248 1984; fax: + 1 780 492 0364.